15.08.2006 Ref.: EURISOL DS/Task5/TN-06-03

Nuclide inventories in Hg-targets Compiled by R.Moormann (FZJ) Contribution to WP5.1, Deliverable D1

K.Bongardt, B.Lensing, R.Moormann, H.Schaal (FZJ) Abstract Information on the radioactive inventory in an Hg-target, as calculated by SNS, ESS and JSNS. Appendix 1 contains a list of about 500 nuclides and their activities expected after 40 y of operation of a 5 MW target. Data for masses < 100 still require some additional examinations by respective computer calculations. Although for the majority of the nuclides with masses > 100 the confidential band is expected to be within of a factor of 2, more experimental validation is advisable.

Detailed calculations on the inventories of Hg-targets were performed at SNS [1], ESS [2] and JSNS [4]. It has to be noted, that former inventory calculations of 1996 for ESS [5] resulted in far lower values for long lived nuclides. This is probably due to insufficient knowledge concerning certain spallation chains at that time (particularly in chains, resulting in Gd-148, Ho-163 and Hg-194); recent recalculations for ESS came to the conclusion, that the SNS data are probably correct [2, 3, 6], except for Ho-163, where the inventory is by a factor of 80 overestimated in PSAR-SNS. It has to be noted, that SNS calculations deal mainly with nuclides of masses > 100 (except tritium); preliminary ESS calculations came to the conclusion, that masses < 100 may not be neglected. Because these examinations for low masses were performed in the final stage of the ESS project, they were not completely finished and require some additional calculation. Further on, measurements on spallation nuclide concentrations in SINQ irradiated mercury are desirable (giving results on intermediate and long lived nuclides only). Concentrations of the following nuclides should be determined in these experiments: HG-194, GD-148, HF-172, HO-163, BA-133, LA-137, PM-145, EU-150, PT-193, AU-195.

The following table (Appendix I) contains the best estimate inventories of about 500 nuclides for 40 y target lifetime (5000 h/y of operation) immediately after shut down; data are based mainly on SNS and ESS calculations. The uncertainty margin has to be assumed for most (70 %) nuclides with masses > 100 - following SNS estimations - with a factor of 2. Volatile nuclides are presented in red colour, Hg-nuclides in blue.

Nuclide inventories in Hg targets: Compiled by R.Moormann/FZJ

15.08.2006)

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References [1] SNS Preliminary Safety Analysis Report (PSAR), Feb. 28 (2000), US DOE Contract No. AC05-96OR22464 [2] B. Lensing, Untersuchung sicherheitstechnisch relevanter nuklearer Parameter einer hochintensiven Spallationquelle im MW Bereich am Beispiel des Referenzentwurfes der Europäischen Spallationsneutonenquelle (ESS). PhD thesis, University of Wuppertal, Germany, 2004 [3] H.Schaal, B.Lensing, private communication (2003) [4] F Maekawa, M Harada, M Teshigawara, T Kai, Y Kiyanagi: personal communication, 2002 [5] The ESS technical study. ESS-96-53-M (1996) [6] R.Moormann et al.: Status of Safety Analyses for the ESS Target. Proc. 1st SAFERIBWorkshop, Report CERN-2003-004 (2003).

Nuclide inventories in Hg targets: Compiled by R.Moormann/FZJ

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Appendix I:

t1/2/d

t1/2/y

Activity/GBq

Nuclide

t1/2/s

H3 C14 Si32 P32 Cl36 Ar39 Ar42 K42 Ca41 Sc44 Ti44 Fe60 Co60 Ni63 Se79 Kr81 Sr90 Y90 Zr93 Nb91 Nb93m Nb94 Mo93 Tc97

3.89E+008 1.81E+011 5.43E+009 1.21E+006 9.50E+012 8.52E+009 1.04E+009 4.32E+004 3.15E+012 1.44E+004 1.55E+009 4.10E+013 1.66E+008 3.11E+009 2.05E+013 7.22E+012 9.16E+008 2.31E+005 4.75E+013 2.14E+010 5.09E+008 7.26E+011 1.26E+011 8.20E+013

4.50E+003 1.23E+001 2.09E+006 5.73E+003 6.28E+004 1.72E+002 1.40E+001 3.84E-002 1.10E+008 3.01E+005 9.86E+004 2.70E+002 1.20E+004 3.29E+001 5.00E-001 1.37E-003 3.65E+007 1.00E+005 1.67E-001 4.58E-004 1.79E+004 4.90E+001 4.75E+008 1.30E+006 1.92E+003 5.26E+000 3.60E+004 9.86E+001 2.37E+008 6.49E+005 8.36E+007 2.29E+005 1.06E+004 2.90E+001 2.67E+000 7.32E-003 5.50E+008 1.51E+006 2.48E+005 6.80E+002 5.89E+003 1.61E+001 8.40E+006 2.30E+004 1.46E+006 4.00E+003 9.49E+008 2.60E+006

1.60E+001 1.50E+003 1.50E+003 5.00E-001 1.60E+003 9.60E+003 9.60E+003 1.10E+000 1.30E+002 1.30E+002 3.50E-001 1.80E+005 8.00E+003 2.10E+000 5.50E+001 9.50E+003 9.50E+003 5.00E-001 4.01E+005 4.05E+001 1.50E+001 4.00E+001 1.50E-001

Tc98 Tc99 Rh101 Pd107 Ag109m Cd109 Cd113m Cd115 In110 In111 In112 In114 In115m In116m In117 Sn113 Sn121m Sb113 Sb115 Sb116 Sb117 Sb118 Sb119 Sb120 Sb122 Sb124 Sb125 Te117 Te118

1.32E+014 6.66E+012 1.04E+008 2.05E+014 3.96E+001 4.01E+007 4.45E+008 1.93E+005 1.76E+004 2.45E+005 1.24E+003 7.20E+001 1.62E+004 3.39E+002 2.63E+003 9.94E+006 1.74E+009 4.00E+002 1.93E+003 9.50E+002 1.01E+004 2.16E+002 1.37E+005 9.50E+002 2.33E+005 5.20E+006 8.61E+007 3.71E+003 5.18E+005

1.53E+009 7.71E+007 1.20E+003 2.37E+009 4.58E-004 4.64E+002 5.15E+003 2.23E+000 2.04E-001 2.83E+000 1.43E-002 8.33E-004 1.87E-001 3.92E-003 3.04E-002 1.15E+002 2.01E+004 4.63E-003 2.23E-002 1.10E-002 1.17E-001 2.50E-003 1.59E+000 1.10E-002 2.70E+000 6.02E+001 9.96E+002 4.29E-002 6.00E+000

1.50E-001 3.50E+000 3.13E+002 1.50E-001 3.13E+002 3.13E+002 4.50E-001 3.13E+002 3.13E+002 6.25E+002 3.13E+002 6.25E+002 3.13E+002 6.25E+002 3.13E+002 6.25E+002 4.50E+002 6.25E+002 1.56E+003 9.38E+002 4.38E+003 4.07E+003 4.07E+003 2.81E+003 6.25E+002 3.13E+002 9.29E+002 2.18E+003 2.50E+003

4.19E+006 2.11E+005 3.29E+000 6.49E+006 1.25E-006 1.27E+000 1.41E+001 6.11E-003 5.59E-004 7.75E-003 3.92E-005 2.28E-006 5.12E-004 1.07E-005 8.33E-005 3.15E-001 5.51E+001 1.27E-005 6.11E-005 3.01E-005 3.21E-004 6.85E-006 4.36E-003 3.01E-005 7.40E-003 1.65E-001 2.73E+000 1.18E-004 1.64E-002

Nuclide inventories in Hg targets: Compiled by R.Moormann/FZJ

5.55E+005

15.08.2006)

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Nuclide

t1/2/s

t1/2/d

t1/2/y

Activity/GBq

Te119 Te121 Te125m I119 I120 I121 I122 I123 I124 I125 I126 I128 I129 Xe119 Xe120 Xe121 Xe122 Xe123 Xe125 Xe127 Cs120 Cs123 Cs124 Cs125 Cs126 Cs127 Cs128 Cs129 Cs130 Cs131 Cs132 Cs136 Ba123 Ba124 Ba125 Ba126 Ba127 Ba128 Ba129 Ba131 Ba133 Ba136m La126 La127 La128 La129 La130 La131 La132 La133 La134 La135 La136

5.78E+004 1.45E+006 5.01E+006 1.15E+003 4.86E+003 7.63E+003 2.18E+002 4.75E+004 3.61E+005 5.19E+006 1.12E+006 1.50E+003 4.95E+014 3.48E+002 2.40E+003 2.40E+003 7.24E+004 7.49E+003 6.12E+004 3.14E+006 6.06E+001 3.53E+002 3.08E+001 2.70E+003 9.85E+001 2.25E+004 2.17E+002 1.16E+005 1.80E+003 8.37E+005 5.59E+005 1.14E+006 1.62E+002 7.10E+002 2.10E+002 6.01E+003 7.62E+002 2.10E+005 7.99E+003 1.02E+006 3.32E+008 3.10E-001 6.00E+001 2.30E+002 3.00E+002 6.96E+002 5.22E+002 3.54E+003 1.73E+004 1.41E+004 3.87E+002 7.02E+004 5.92E+002

6.69E-001 1.68E+001 5.80E+001 1.33E-002 5.63E-002 8.83E-002 2.52E-003 5.50E-001 4.18E+000 6.01E+001 1.30E+001 1.74E-002 5.73E+009 4.03E-003 2.78E-002 2.78E-002 8.38E-001 8.67E-002 7.08E-001 3.64E+001 7.01E-004 4.08E-003 3.56E-004 3.13E-002 1.14E-003 2.60E-001 2.51E-003 1.34E+000 2.08E-002 9.69E+000 6.47E+000 1.32E+001 1.88E-003 8.22E-003 2.43E-003 6.96E-002 8.82E-003 2.43E+000 9.25E-002 1.18E+001 3.84E+003 3.59E-006 6.94E-004 2.66E-003 3.47E-003 8.06E-003 6.04E-003 4.10E-002 2.00E-001 1.63E-001 4.48E-003 8.13E-001 6.85E-003

1.83E-003 4.60E-002 1.59E-001 3.64E-005 1.54E-004 2.42E-004 6.90E-006 1.51E-003 1.15E-002 1.65E-001 3.56E-002 4.77E-005 1.57E+007 1.10E-005 7.62E-005 7.62E-005 2.30E-003 2.38E-004 1.94E-003 9.97E-002 1.92E-006 1.12E-005 9.75E-007 8.58E-005 3.12E-006 7.12E-004 6.88E-006 3.67E-003 5.70E-005 2.65E-002 1.77E-002 3.62E-002 5.15E-006 2.25E-005 6.66E-006 1.91E-004 2.42E-005 6.66E-003 2.53E-004 3.23E-002 1.05E+001 9.84E-009 1.90E-006 7.29E-006 9.51E-006 2.21E-005 1.65E-005 1.12E-004 5.48E-004 4.47E-004 1.23E-005 2.23E-003 1.88E-005

3.13E+003 5.00E+003 1.44E+002 1.25E+003 1.87E+003 3.76E+003 5.31E+003 6.88E+003 3.13E+003 1.37E+004 6.25E+002 6.25E+002 1.64E-003 6.25E+002 6.25E+002 3.13E+002 2.18E+003 3.76E+003 1.06E+004 2.68E+004 3.13E+002 1.56E+003 3.44E+003 3.76E+003 1.00E+004 2.22E+004 3.48E+004 3.77E+004 7.20E+003 4.79E+004 1.25E+003 3.13E+002 3.13E+002 9.38E+002 3.13E+002 6.25E+003 1.16E+004 2.26E+004 2.98E+004 4.44E+004 1.50E+004 5.00E+001 3.13E+002 3.13E+003 9.07E+003 1.53E+004 2.26E+004 3.09E+004 2.98E+004 1.69E+004 2.16E+004 3.76E+004 4.07E+003

Nuclide inventories in Hg targets: Compiled by R.Moormann/FZJ

15.08.2006)

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Nuclide

t1/2/s

t1/2/d

t1/2/y

Activity/GBq

La137 La140 Ce130 Ce131 Ce132 Ce133 Ce134 Ce135 Ce137 Ce139 Ce141 Ce142 Pr132 Pr133 Pr134 Pr135 Pr136 Pr137 Pr138 Pr139 Pr140 Pr142 Pr143 Nd135 Nd136 Nd137 Nd138 Nd139 Nd140 Nd141 Nd147 Pm136 Pm137 Pm138 Pm139 Pm140 Pm141 Pm142 Pm143 Pm144 Pm145 Pm146 Pm147 Pm148 Pm150 Pm153 Sm138 Sm139 Sm140 Sm141 Sm142 Sm143 Sm145

1,89E+012 1,45E+005 8,63E+004 6,00E+002 8,63E+004 1,76E+004 2,73E+005 6,37E+004 3,24E+004 1,19E+007 2,81E+006 1,58E+024 8,63E+004 3,90E+002 1,02E+003 1,44E+003 7,86E+002 4,61E+003 8,73E+001 1,59E+004 2,03E+002 6,89E+004 1,18E+006 7,40E+002 3,04E+003 2,31E+003 1,81E+004 1,78E+003 2,91E+005 8,99E+003 9,50E+005 1,07E+002 1,44E+002 1,00E+001 2,49E+002 9,16E+000 1,25E+003 4,05E+001 2,29E+007 3,14E+007 5,58E+008 1,75E+008 8,26E+007 4,64E+005 9,68E+003 3,24E+002 1,80E+002 1,54E+002 8,90E+002 6,12E+002 4,35E+003 5,30E+002 2,94E+007

2,19E+007 1,68E+000 9,99E-001 6,94E-003 9,99E-001 2,04E-001 3,16E+000 7,37E-001 3,75E-001 1,38E+002 3,25E+001 1,83E+019 9,99E-001 4,51E-003 1,18E-002 1,67E-002 9,10E-003 5,33E-002 1,01E-003 1,84E-001 2,35E-003 7,97E-001 1,36E+001 8,56E-003 3,52E-002 2,67E-002 2,10E-001 2,06E-002 3,37E+000 1,04E-001 1,10E+001 1,24E-003 1,67E-003 1,16E-004 2,88E-003 1,06E-004 1,45E-002 4,69E-004 2,65E+002 3,63E+002 6,46E+003 2,02E+003 9,56E+002 5,37E+000 1,12E-001 3,75E-003 2,08E-003 1,78E-003 1,03E-002 7,08E-003 5,04E-002 6,13E-003 3,40E+002

6,00E+004 4,60E-003 2,74E-003 1,90E-005 2,74E-003 5,59E-004 8,66E-003 2,02E-003 1,03E-003 3,78E-001 8,90E-002 5,01E+016 2,74E-003 1,24E-005 3,23E-005 4,58E-005 2,49E-005 1,46E-004 2,77E-006 5,04E-004 6,44E-006 2,18E-003 3,73E-002 2,35E-005 9,64E-005 7,32E-005 5,75E-004 5,64E-005 9,23E-003 2,85E-004 3,01E-002 3,40E-006 4,58E-006 3,18E-007 7,89E-006 2,90E-007 3,97E-005 1,28E-006 7,26E-001 9,95E-001 1,77E+001 5,53E+000 2,62E+000 1,47E-002 3,07E-004 1,03E-005 5,70E-006 4,88E-006 2,82E-005 1,94E-005 1,38E-004 1,68E-005 9,32E-001

2,66E+001 3,13E+002 8,12E+003 1,25E+004 1,66E+004 1,12E+004 1,72E+004 3,53E+004 7,66E+004 9,97E+004 3,13E+002 6,20E-008 4,07E+003 4,07E+003 6,57E+003 2,53E+004 5,66E+004 7,12E+004 8,20E+004 9,88E+004 1,20E+005 6,25E+002 3,13E+002 7,20E+003 2,59E+004 4,85E+004 6,20E+004 9,07E+004 1,15E+005 1,43E+005 6,25E+002 6,88E+003 1,94E+004 3,48E+004 6,31E+004 9,44E+004 1,28E+005 1,56E+005 1,71E+005 1,34E+004 1,15E+005 1,44E+003 1,56E+003 1,25E+003 6,25E+002 3,13E+002 9,38E+002 2,09E+004 4,27E+004 7,60E+004 1,25E+005 1,46E+005 2,00E+005

Nuclide inventories in Hg targets: Compiled by R.Moormann/FZJ

15.08.2006)

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Nuclide

t1/2/s

t1/2/d

t1/2/y

Activity/GBq

Sm147 Sm151 Sm153 Eu141 Eu142 Eu143 Eu144 Eu145 Eu146 Eu147 Eu148 Eu149 Eu150 Eu152 Eu154 Eu155 Eu156 Gd143 Gd144 Gd145 Gd146 Gd147 Gd148 Gd149 Gd150 Gd151 Gd152 Gd153 Tb146 Tb147 Tb148 Tb149 Tb150 Tb151 Tb152 Tb153 Tb154 Tb155 Tb156 Tb157 Tb158 Dy148 Dy149 Dy150 Dy151 Dy152 Dy153 Dy154 Dy155 Dy157 Dy159 Ho150 Ho151

3.34E+018 2.80E+009 1.68E+005 4.00E+001 2.40E+000 1.58E+002 1.02E+001 5.12E+005 3.97E+005 2.07E+006 4.71E+006 8.04E+006 1.08E+009 4.20E+008 2.71E+008 1.56E+008 1.31E+006 3.90E+001 2.70E+002 1.38E+003 4.17E+006 1.37E+005 2.35E+009 8.10E+005 5.64E+013 1.07E+007 3.40E+021 2.09E+007 8.00E+000 5.90E+003 3.60E+003 1.49E+004 1.25E+004 6.34E+004 6.30E+004 2.02E+005 7.74E+004 4.60E+005 4.62E+005 3.10E+009 5.69E+009 1.86E+002 2.54E+002 4.30E+002 1.07E+003 8.54E+003 2.30E+004 8.99E+013 3.60E+004 2.93E+004 1.24E+007 8.81E+001 3.52E+001

3.87E+013 3.24E+004 1.95E+000 4.63E-004 2.78E-005 1.83E-003 1.18E-004 5.93E+000 4.59E+000 2.40E+001 5.45E+001 9.31E+001 1.25E+004 4.86E+003 3.14E+003 1.81E+003 1.52E+001 4.51E-004 3.13E-003 1.60E-002 4.83E+001 1.59E+000 2.72E+004 9.38E+000 6.53E+008 1.24E+002 3.94E+016 2.42E+002 9.26E-005 6.83E-002 4.17E-002 1.72E-001 1.45E-001 7.34E-001 7.29E-001 2.34E+000 8.96E-001 5.32E+000 5.35E+000 3.59E+004 6.59E+004 2.15E-003 2.94E-003 4.98E-003 1.24E-002 9.88E-002 2.66E-001 1.04E+009 4.17E-001 3.39E-001 1.44E+002 1.02E-003 4.07E-004

1.06E+011 8.88E+001 5.34E-003 1.27E-006 7.62E-008 5.01E-006 3.23E-007 1.62E-002 1.26E-002 6.58E-002 1.49E-001 2.55E-001 3.42E+001 1.33E+001 8.60E+000 4.96E+000 4.16E-002 1.24E-006 8.58E-006 4.38E-005 1.32E-001 4.36E-003 7.45E+001 2.57E-002 1.79E+006 3.40E-001 1.08E+014 6.63E-001 2.54E-007 1.87E-004 1.14E-004 4.71E-004 3.97E-004 2.01E-003 2.00E-003 6.41E-003 2.45E-003 1.46E-002 1.47E-002 9.84E+001 1.81E+002 5.89E-006 8.05E-006 1.36E-005 3.40E-005 2.71E-004 7.29E-004 2.85E+006 1.14E-003 9.29E-004 3.95E-001 2.79E-006 1.12E-006

3.42E-005 1.87E+002 3.13E+002 1.75E+004 5.07E+004 7.62E+004 1.22E+005 1.78E+005 1.94E+005 1.65E+005 1.87E+004 1.72E+005 3.57E+003 2.76E+003 5.70E+002 3.11E+002 3.13E+002 1.81E+004 4.03E+004 7.97E+004 1.43E+005 1.31E+005 3.50E+004 1.55E+005 2.15E+000 2.42E+005 3.96E-008 2.98E+005 2.09E+004 5.27E+004 1.24E+005 1.28E+005 1.46E+005 2.20E+005 2.94E+005 2.85E+005 4.35E+004 3.15E+005 1.12E+004 4.03E+004 3.31E+002 6.22E+004 6.14E+004 1.01E+005 1.62E+005 2.29E+005 2.33E+005 6.20E-001 2.90E+005 3.00E+005 2.42E+005 2.59E+004 7.70E+004

Nuclide inventories in Hg targets: Compiled by R.Moormann/FZJ

15.08.2006)

6

Nuclide

t1/2/s

Ho152 Ho153 Ho154 Ho155 Ho156 Ho157 Ho158 Ho159 Ho160 Ho161 Ho162 Ho163 Er151 Er152 Er153 Er154 Er155 Er156 Er157 Er158 Er159 Er160 Er161 Er163 Er165 Tm154 Tm155 Tm156 Tm157 Tm158 Tm159 Tm160 Tm161 Tm162 Tm163 Tm164 Tm165 Tm166 Tm167 Tm168 Yb155 Yb156 Yb157 Yb158 Yb159 Yb160 Yb161 Yb162 Yb163 Yb164 Yb165 Yb166 Yb167

1.62E+002 1.20E+002 7.10E+002 2.88E+003 3.36E+003 7.56E+002 6.60E+002 1.99E+003 8.63E+004 8.90E+003 8.99E+002 1.44E+011 2.35E+001 1.01E+001 3.71E+001 2.21E+002 3.18E+002 1.17E+003 1.12E+003 8.10E+003 2.16E+003 1.03E+005 1.16E+004 4.50E+003 3.73E+004 8.10E+000 3.40E+001 8.40E+001 2.10E+002 2.41E+002 5.49E+002 5.64E+002 2.28E+003 1.30E+003 6.51E+003 1.20E+002 1.08E+005 2.80E+004 7.98E+005 8.04E+006 1.71E+000 2.61E+001 3.86E+001 9.94E+001 8.40E+001 2.88E+002 2.52E+002 1.13E+003 6.63E+002 4.54E+003 5.94E+002 2.04E+005 1.05E+003

t1/2/d

t1/2/y

1.88E-003 5.15E-006 1.39E-003 3.81E-006 8.22E-003 2.25E-005 3.33E-002 9.12E-005 3.89E-002 1.07E-004 8.75E-003 2.40E-005 7.64E-003 2.09E-005 2.30E-002 6.30E-005 9.99E-001 2.74E-003 1.03E-001 2.82E-004 1.04E-002 2.85E-005 1.67E+006 4.58E+003 2.72E-004 7.45E-007 1.17E-004 3.21E-007 4.29E-004 1.18E-006 2.56E-003 7.01E-006 3.68E-003 1.01E-005 1.35E-002 3.70E-005 1.30E-002 3.56E-005 9.38E-002 2.57E-004 2.50E-002 6.85E-005 1.19E+000 3.26E-003 1.34E-001 3.67E-004 5.21E-002 1.43E-004 4.32E-001 1.18E-003 9.38E-005 2.57E-007 3.94E-004 1.08E-006 9.72E-004 2.66E-006 2.43E-003 6.66E-006 2.79E-003 7.64E-006 6.35E-003 1.74E-005 6.53E-003 1.79E-005 2.64E-002 7.23E-005 1.51E-002 4.14E-005 7.54E-002 2.07E-004 1.39E-003 3.81E-006 1.25E+000 3.42E-003 3.24E-001 8.88E-004 9.24E+000 2.53E-002 9.31E+001 2.55E-001 1.98E-005 5.42E-008 3.02E-004 8.27E-007 4.47E-004 1.22E-006 1.15E-003 3.15E-006 9.72E-004 2.66E-006 3.33E-003 9.12E-006 2.92E-003 8.00E-006 1.31E-002 3.59E-005 7.67E-003 2.10E-005 5.25E-002 1.44E-004 6.88E-003 1.88E-005 2.36E+000 6.47E-003 1.22E-002 3.34E-005

Nuclide inventories in Hg targets: Compiled by R.Moormann/FZJ

Activity/GBq 1.15E+005 1.30E+005 1.89E+005 2.20E+005 2.48E+005 2.68E+005 3.00E+005 2.37E+005 2.13E+005 1.81E+005 9.38E+002 9.60E+002 1.34E+004 3.48E+004 5.79E+004 7.44E+004 9.62E+004 1.23E+005 1.68E+005 2.39E+005 2.09E+005 2.02E+005 1.76E+005 1.48E+005 2.05E+005 1.09E+004 2.26E+004 3.81E+004 5.35E+004 1.13E+005 1.32E+005 1.42E+005 1.51E+005 2.48E+005 1.42E+005 2.55E+005 2.04E+005 4.03E+005 3.66E+005 6.25E+002 3.76E+003 7.51E+003 2.22E+004 2.81E+004 3.44E+004 6.31E+004 8.25E+004 1.87E+005 1.05E+005 2.35E+005 1.92E+005 3.98E+005 3.64E+005

15.08.2006)

7

Nuclide

t1/2/s

t1/2/d

t1/2/y

Activity/GBq

Yb169 Lu162 Lu164 Lu165 Lu166 Lu167 Lu168 Lu169 Lu170 Lu171 Lu172 Lu173 Lu174 Lu176 Hf159 Hf160 Hf161 Hf166 Hf167 Hf168 Hf169 Hf170 Hf171 Hf172 Hf173 Hf175 Ta166 Ta167 Ta168 Ta169 Ta170 Ta171 Ta172 Ta173 Ta174 Ta175 Ta176 Ta177 Ta178 Ta179 Ta182 Ta183 W165 W166 W170 W171 W172 W173 W174 W175 W176 W177 W178

2.76E+006 8.22E+001 1.88E+002 6.44E+002 4.59E+002 3.09E+003 3.30E+002 1.23E+005 1.73E+005 7.12E+005 5.79E+005 4.32E+007 1.05E+008 1.14E+018 5.60E+000 1.20E+001 1.70E+001 4.06E+002 1.23E+002 8.63E+004 1.94E+002 5.76E+004 4.36E+004 5.90E+007 8.64E+004 6.05E+006 3.44E+001 8.63E+004 8.63E+004 2.94E+002 4.06E+002 1.40E+003 2.21E+003 1.13E+004 4.25E+003 3.78E+004 2.91E+004 2.04E+005 5.59E+002 5.58E+007 9.94E+006 4.41E+005 5.10E+000 1.60E+001 8.63E+004 8.63E+004 4.00E+002 8.63E+004 1.76E+003 2.04E+003 8.32E+003 8.10E+003 1.87E+006

3.20E+001 9.51E-004 2.18E-003 7.45E-003 5.31E-003 3.58E-002 3.82E-003 1.42E+000 2.00E+000 8.24E+000 6.70E+000 5.00E+002 1.21E+003 1.32E+013 6.48E-005 1.39E-004 1.97E-004 4.70E-003 1.42E-003 9.99E-001 2.25E-003 6.67E-001 5.05E-001 6.83E+002 1.00E+000 7.00E+001 3.98E-004 9.99E-001 9.99E-001 3.40E-003 4.70E-003 1.62E-002 2.56E-002 1.31E-001 4.92E-002 4.38E-001 3.37E-001 2.36E+000 6.47E-003 6.46E+002 1.15E+002 5.10E+000 5.90E-005 1.85E-004 9.99E-001 9.99E-001 4.63E-003 9.99E-001 2.04E-002 2.36E-002 9.63E-002 9.38E-002 2.16E+001

8.77E-002 2.61E-006 5.97E-006 2.04E-005 1.45E-005 9.81E-005 1.05E-005 3.89E-003 5.48E-003 2.26E-002 1.84E-002 1.37E+000 3.32E+000 3.62E+010 1.78E-007 3.81E-007 5.40E-007 1.29E-005 3.89E-006 2.74E-003 6.16E-006 1.83E-003 1.38E-003 1.87E+000 2.74E-003 1.92E-001 1.09E-006 2.74E-003 2.74E-003 9.32E-006 1.29E-005 4.44E-005 7.01E-005 3.59E-004 1.35E-004 1.20E-003 9.23E-004 6.47E-003 1.77E-005 1.77E+000 3.15E-001 1.40E-002 1.62E-007 5.07E-007 2.74E-003 2.74E-003 1.27E-005 2.74E-003 5.59E-005 6.47E-005 2.64E-004 2.57E-004 5.92E-002

3.46E+005 7.88E+004 1.50E+005 1.41E+005 3.74E+005 3.52E+005 3.96E+005 3.40E+005 5.99E+005 4.44E+005 7.31E+005 3.11E+005 1.54E+003 3.61E-007 6.25E+002 1.25E+003 8.75E+003 2.48E+005 2.79E+005 3.46E+005 3.13E+005 5.81E+005 4.37E+005 7.27E+005 3.07E+005 7.05E+005 1.06E+005 1.42E+005 2.20E+005 2.13E+005 5.07E+005 3.96E+005 7.01E+005 2.90E+005 7.34E+005 7.01E+005 6.99E+005 6.70E+005 9.01E+005 8.86E+005 3.13E+002 3.13E+002 5.94E+003 2.31E+004 2.85E+005 2.13E+005 5.68E+005 2.02E+005 6.70E+005 6.60E+005 6.72E+005 6.55E+005 8.88E+005

Nuclide inventories in Hg targets: Compiled by R.Moormann/FZJ

15.08.2006)

8

Nuclide

t1/2/s

t1/2/d

t1/2/y

Activity/GBq

W179 W179m W181 W183m W185 W188 Re170 Re172 Re174 Re175 Re176 Re177 Re178 Re179 Re180 Re181 Re182 Re183 Re184 Re186 Re188 Re190 Re192 Os169 Os170 Os171 Os172 Os173 Os174 Os175 Os176 Os177 Os178 Os179 Os180 Os181 Os182 Os183 Os183m Os185 Os189m Os191 Os193 Os196 Ir172 Ir173 Ir174 Ir175 Ir176 Ir177 Ir178 Ir179 Ir180

2.25E+003 3.84E+002 1.05E+007 5.20E+000 6.49E+006 6.00E+006 8.00E+000 1.50E+001 1.38E+002 8.63E+004 3.40E+002 8.40E+002 7.92E+002 1.17E+003 1.46E+002 7.20E+004 2.31E+005 6.05E+006 3.28E+006 3.27E+005 6.12E+004 1.86E+002 1.60E+001 3.50E+000 7.10E+000 8.00E+000 1.90E+001 1.60E+001 4.40E+001 8.63E+004 1.80E+002 2.10E+002 3.05E+002 3.90E+002 1.29E+003 1.62E+002 7.96E+004 4.68E+004 3.56E+004 8.09E+006 1.73E+004 1.33E+006 1.10E+005 2.09E+003 8.63E+004 3.00E+000 4.00E+000 4.50E+000 8.63E+004 2.10E+001 1.20E+001 8.63E+004 8.99E+001

2.60E-002 4.44E-003 1.21E+002 6.02E-005 7.51E+001 6.94E+001 9.26E-005 1.74E-004 1.60E-003 9.99E-001 3.94E-003 9.72E-003 9.17E-003 1.35E-002 1.69E-003 8.33E-001 2.67E+000 7.00E+001 3.80E+001 3.78E+000 7.08E-001 2.15E-003 1.85E-004 4.05E-005 8.22E-005 9.26E-005 2.20E-004 1.85E-004 5.09E-004 9.99E-001 2.08E-003 2.43E-003 3.53E-003 4.51E-003 1.49E-002 1.88E-003 9.21E-001 5.42E-001 4.12E-001 9.36E+001 2.00E-001 1.54E+001 1.27E+000 2.42E-002 9.99E-001 3.47E-005 4.63E-005 5.21E-005 9.99E-001 2.43E-004 1.39E-004 9.99E-001 1.04E-003

7.12E-005 1.22E-005 3.32E-001 1.65E-007 2.06E-001 1.90E-001 2.54E-007 4.77E-007 4.38E-006 2.74E-003 1.08E-005 2.66E-005 2.51E-005 3.70E-005 4.63E-006 2.28E-003 7.32E-003 1.92E-001 1.04E-001 1.04E-002 1.94E-003 5.89E-006 5.07E-007 1.11E-007 2.25E-007 2.54E-007 6.03E-007 5.07E-007 1.39E-006 2.74E-003 5.70E-006 6.66E-006 9.67E-006 1.24E-005 4.08E-005 5.15E-006 2.52E-003 1.48E-003 1.13E-003 2.56E-001 5.48E-004 4.22E-002 3.48E-003 6.63E-005 2.74E-003 9.51E-008 1.27E-007 1.43E-007 2.74E-003 6.66E-007 3.81E-007 2.74E-003 2.85E-006

8.82E+005 6.16E+005 9.97E+005 1.66E+002 1.25E+003 3.13E+002 1.13E+005 3.63E+005 5.07E+005 5.33E+005 5.88E+005 5.85E+005 8.38E+005 8.53E+005 9.25E+005 9.86E+005 1.01E+006 1.04E+006 2.41E+004 1.22E+004 9.38E+002 3.13E+002 3.13E+002 1.56E+003 6.25E+003 2.46E+004 5.90E+004 1.01E+005 1.63E+005 2.29E+005 2.85E+005 3.15E+005 5.99E+005 6.77E+005 7.92E+005 8.94E+005 9.51E+005 6.35E+005 4.05E+005 9.82E+005 1.49E+005 3.13E+003 6.25E+002 3.13E+002 1.56E+003 2.50E+003 2.41E+004 5.77E+004 9.51E+004 1.61E+005 2.46E+005 3.22E+005 4.57E+005

Nuclide inventories in Hg targets: Compiled by R.Moormann/FZJ

15.08.2006)

9

Nuclide

t1/2/s

t1/2/d

t1/2/y

Activity/GBq

Ir181 Ir182 Ir183 Ir184 Ir185 Ir186 Ir187 Ir188 Ir189 Ir190 Ir192 Ir194 Ir195 Ir196 Ir197 Ir198 Pt175 Pt176 Pt177 Pt178 Pt179 Pt180 Pt181 Pt182 Pt183 Pt184 Pt185 Pt185m Pt186 Pt187 Pt188 Pt189 Pt191 Pt193 Pt197 Pt197m Pt199 Pt200 Pt201 Au178 Au179 Au181 Au182 Au183 Au184 Au185 Au185m Au186 Au187 Au188 Au189 Au189m Au190

2.94E+002 8.99E+002 3.30E+003 1.09E+004 5.00E+004 5.99E+004 3.78E+004 1.49E+005 1.14E+006 1.02E+006 6.38E+006 6.89E+004 8.99E+003 5.20E+001 3.48E+002 8.00E+000 2.52E+000 8.63E+004 1.10E+001 2.10E+001 4.30E+001 5.20E+001 5.10E+001 1.56E+002 3.90E+002 1.04E+003 4.25E+003 8.63E+004 7.20E+003 8.46E+003 8.81E+005 3.92E+004 2.51E+005 1.60E+009 6.59E+004 5.65E+003 1.85E+003 4.50E+004 1.50E+002 2.60E+000 7.50E+000 1.14E+001 2.10E+001 4.20E+001 5.30E+001 2.60E+002 8.63E+004 6.40E+002 5.04E+002 5.30E+002 1.72E+003 2.76E+002 2.57E+003

3.40E-003 1.04E-002 3.82E-002 1.26E-001 5.79E-001 6.93E-001 4.38E-001 1.73E+000 1.32E+001 1.18E+001 7.38E+001 7.98E-001 1.04E-001 6.02E-004 4.03E-003 9.26E-005 2.92E-005 9.99E-001 1.27E-004 2.43E-004 4.98E-004 6.02E-004 5.90E-004 1.81E-003 4.51E-003 1.20E-002 4.92E-002 9.99E-001 8.33E-002 9.79E-002 1.02E+001 4.54E-001 2.91E+000 1.85E+004 7.63E-001 6.54E-002 2.14E-002 5.21E-001 1.74E-003 3.01E-005 8.68E-005 1.32E-004 2.43E-004 4.86E-004 6.13E-004 3.01E-003 9.99E-001 7.41E-003 5.83E-003 6.13E-003 1.99E-002 3.19E-003 2.97E-002

9.32E-006 2.85E-005 1.05E-004 3.45E-004 1.59E-003 1.90E-003 1.20E-003 4.74E-003 3.62E-002 3.23E-002 2.02E-001 2.19E-003 2.85E-004 1.65E-006 1.10E-005 2.54E-007 8.00E-008 2.74E-003 3.48E-007 6.66E-007 1.36E-006 1.65E-006 1.62E-006 4.96E-006 1.24E-005 3.29E-005 1.35E-004 2.74E-003 2.28E-004 2.68E-004 2.79E-002 1.24E-003 7.97E-003 5.07E+001 2.09E-003 1.79E-004 5.86E-005 1.43E-003 4.77E-006 8.25E-008 2.38E-007 3.62E-007 6.66E-007 1.33E-006 1.68E-006 8.25E-006 2.74E-003 2.03E-005 1.60E-005 1.68E-005 5.45E-005 8.74E-006 8.14E-005

5.88E+005 7.22E+005 8.10E+005 9.19E+005 9.01E+005 1.07E+006 1.32E+006 1.77E+006 1.98E+006 6.07E+004 3.13E+004 1.37E+004 1.34E+004 7.81E+003 3.76E+003 1.87E+003 3.61E+003 1.03E+004 2.37E+004 4.00E+004 6.77E+004 1.22E+005 2.16E+005 3.27E+005 4.26E+005 5.42E+005 5.92E+005 3.46E+004 8.60E+005 1.18E+006 1.65E+006 1.89E+006 2.42E+006 1.05E+006 1.02E+005 1.87E+003 5.03E+004 3.61E+004 1.18E+004 2.18E+003 7.96E+003 3.66E+004 7.33E+004 1.06E+005 1.73E+005 2.11E+005 3.46E+004 4.48E+005 7.36E+005 1.15E+006 7.84E+005 6.85E+005 1.85E+006

Nuclide inventories in Hg targets: Compiled by R.Moormann/FZJ

15.08.2006)

10

Nuclide

t1/2/s

Au191 Au191m Au192 Au193 Au194 Au195 Au195m Au196 Au197m Au198 Au199 Au200 Au201 Au202 Au203 Au204 Hg180 Hg181 Hg182 Hg183 Hg184 Hg185 Hg186 Hg187 Hg188 Hg189 Hg190 Hg191 Hg192 Hg193 Hg194 Hg195 Hg197 Hg203 Hg205 Tl184 Tl186 Tl188 Tl189 Tl190 Tl191 Tl192 Tl193 Tl194 Tl195 Tl195m Tl196 Tl197 Tl198 Tl199 Tl200 Tl201 Tl202

1.14E+004 9.16E-001 1.78E+004 6.35E+004 1.37E+005 1.61E+007 3.05E+001 5.34E+005 7.80E+000 2.33E+005 2.71E+005 2.90E+003 1.56E+003 2.88E+001 5.30E+001 3.98E+001 3.00E+000 3.60E+000 1.13E+001 8.81E+000 3.06E+001 4.90E+001 8.28E+001 1.44E+002 1.95E+002 4.56E+002 1.20E+003 2.90E+003 1.75E+004 1.37E+004 1.64E+010 3.56E+004 2.31E+005 4.03E+006 3.12E+002 1.10E+001 2.75E+001 7.08E+001 1.38E+002 1.56E+002 8.63E+004 6.48E+002 1.30E+003 1.98E+003 4.17E+003 3.60E+000 6.63E+003 1.02E+004 1.91E+004 2.67E+004 9.42E+004 2.63E+005 1.05E+006

t1/2/d

t1/2/y

1.32E-001 3.62E-004 1.06E-005 2.90E-008 2.06E-001 5.64E-004 7.35E-001 2.01E-003 1.58E+000 4.33E-003 1.86E+002 5.10E-001 3.53E-004 9.67E-007 6.18E+000 1.69E-002 9.03E-005 2.47E-007 2.70E+000 7.40E-003 3.14E+000 8.60E-003 3.36E-002 9.21E-005 1.81E-002 4.96E-005 3.33E-004 9.12E-007 6.13E-004 1.68E-006 4.61E-004 1.26E-006 3.47E-005 9.51E-008 4.17E-005 1.14E-007 1.31E-004 3.59E-007 1.02E-004 2.79E-007 3.54E-004 9.70E-007 5.67E-004 1.55E-006 9.58E-004 2.62E-006 1.67E-003 4.58E-006 2.26E-003 6.19E-006 5.28E-003 1.45E-005 1.39E-002 3.81E-005 3.36E-002 9.21E-005 2.03E-001 5.56E-004 1.59E-001 4.36E-004 1.90E+005 5.21E+002 4.12E-001 1.13E-003 2.67E+000 7.32E-003 4.66E+001 1.28E-001 3.61E-003 9.89E-006 1.27E-004 3.48E-007 3.18E-004 8.71E-007 8.19E-004 2.24E-006 1.60E-003 4.38E-006 1.81E-003 4.96E-006 9.99E-001 2.74E-003 7.50E-003 2.05E-005 1.50E-002 4.11E-005 2.29E-002 6.27E-005 4.83E-002 1.32E-004 4.17E-005 1.14E-007 7.67E-002 2.10E-004 1.18E-001 3.23E-004 2.21E-001 6.05E-004 3.09E-001 8.47E-004 1.09E+000 2.99E-003 3.04E+000 8.33E-003 1.22E+001 3.34E-002

Nuclide inventories in Hg targets: Compiled by R.Moormann/FZJ

Activity/GBq 2.16E+006 1.25E+006 2.55E+006 2.87E+006 1.04E+006 4.16E+006 8.40E+004 9.45E+005 6.18E+001 1.25E+006 1.37E+006 9.25E+005 9.58E+005 2.24E+005 1.96E+005 2.78E+004 1.56E+003 4.38E+003 6.57E+003 1.19E+004 2.22E+004 3.63E+004 9.47E+004 1.94E+005 4.44E+005 6.85E+005 9.92E+005 1.25E+006 1.67E+006 1.94E+006 1.41E+005 3.24E+006 2.16E+007 1.54E+007 6.66E+005 6.25E+002 2.18E+003 2.81E+004 6.53E+004 1.30E+005 1.66E+005 2.16E+005 2.76E+005 3.31E+005 3.74E+005 3.76E+003 4.22E+005 4.85E+005 4.90E+005 4.50E+005 3.44E+005 2.44E+005 1.33E+005

15.08.2006)

11

Nuclide Tl204 Pb188 Pb189 Pb190 Pb191 Pb192 Pb193 Pb194 Pb195 Pb196 Pb197 Pb198 Pb199

t1/2/s

t1/2/d

t1/2/y

1.19E+008 1.38E+003 3.78E+000 2.45E+001 2.84E-004 7.78E-007 5.10E+001 5.90E-004 1.62E-006 7.20E+001 8.33E-004 2.28E-006 7.98E+001 9.24E-004 2.53E-006 2.10E+002 2.43E-003 6.66E-006 3.48E+002 4.03E-003 1.10E-005 7.20E+002 8.33E-003 2.28E-005 8.99E+002 1.04E-002 2.85E-005 2.22E+003 2.57E-002 7.04E-005 6.00E+002 6.94E-003 1.90E-005 8.61E+003 9.96E-002 2.73E-004 5.40E+003 6.25E-002 1.71E-004

Nuclide inventories in Hg targets: Compiled by R.Moormann/FZJ

Activity/GBq 2.16E+004 3.13E+002 3.13E+002 1.56E+003 2.18E+003 3.76E+003 3.13E+003 1.87E+003 3.76E+003 6.25E+002 1.56E+003 3.13E+002 1.25E+003

15.08.2006)

12